
Gender:Male
Date of Birth:1989-03-31
Alma Mater:东北大学
Education Level:With Certificate of Graduation for Doctorate Study
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Title of Paper:Wang, Y., Du, T., Qiu, Z., Song, Y., Che, S., & Fang, X. (2018). CO2 adsorption on polyethylenimine-modified ZSM-5 zeolite synthesized from rice husk ash. Materials Chemistry and Physics, 207, 105-113.
Summary:Mesoporous ZSM-5 zeolite as the adsorbent supporting material was synthesized from rice husk ash (RHA), and then impregnated with polyethylenimine (PEI) for amine functional modification. A series of adsorbents (ZSM-5-PEI-X) with different PEI loading ratios were characterized by XRD, FTIR, TGA/DTG, nitrogen adsorption-desorption, SEM and EDX techniques. The measurement of the adsorption capacity at different temperatures was indicated that ZSM-5-PEI-30 had the highest adsorption capacity at 120 °C (1.96 mmol/g). The experimental data were fitted by adsorption kinetic models and isotherm models, indicated that fractional-order model and the Dual-site langmuir model can be used to describe the adsorption mechanism and predict the adsorption performance. The high CO2 adsorption selectivity and regeneration stability suggested that this adsorbent is a potential candidate in the adsorption and separation of CO2 in industrial flue gas.
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